I think it should be a day time, which could serve the region better. 11023/4 CSTM-KOP Sahyadri express is excellent overnight connection between Pune (Dep 22:00) & KOP (arr 6:OO) and reverse timing (KOP-Dep 22:50 Pune arr 6:50). Moreover, this train runs with just 17 coaches with plenty of scope for augmentation to meet additional demand.
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On the other hand, a convenient day time intercity connecting the region with Pune is lacking. An Intercity with following abstract timings should be a nice option:
Pune...
more... dep.6:30 KOP arr. 13:30 & in return direction,
KOP dep. 14:30- Pune arr. 21:30